Spin-Reorientation-Driven Linear Magnetoelectric Effect in Topological Antiferromagnet Cu3TeO6

Virna Kisiček, Damir Dominko, Matija Čulo, Željko Rapljenović, Marko Kuveždić, Martina Dragičević, Helmuth Berger, Xavier Rocquefelte, Mirta Herak, and Tomislav Ivek
Phys. Rev. Lett. 132, 096701 – Published 26 February 2024

Abstract

The search for new materials for energy-efficient electronic devices has gained unprecedented importance. Among the various classes of magnetic materials driving this search are antiferromagnets, magnetoelectrics, and systems with topological spin excitations. Cu3TeO6 is a material that belongs to all three of these classes. Combining static electric polarization and magnetic torque measurements with phenomenological simulations we demonstrate that magnetic-field-induced spin reorientation needs to be taken into account to understand the linear magnetoelectric effect in Cu3TeO6. Our calculations reveal that the magnetic field pushes the system from the nonpolar ground state to the polar magnetic structures. However, nonpolar structures only weakly differing from the obtained polar ones exist due to the weak effect that the field-induced breaking of some symmetries has on the calculated structures. Among those symmetries is the PT (1¯) symmetry, preserved for Dirac points found in Cu3TeO6. Our findings establish Cu3TeO6 as a promising playground to study the interplay of spintronics-related phenomena.

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  • Received 16 November 2022
  • Revised 11 December 2023
  • Accepted 5 January 2024

DOI:https://doi.org/10.1103/PhysRevLett.132.096701

© 2024 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Virna Kisiček1,2,*, Damir Dominko1, Matija Čulo1, Željko Rapljenović1, Marko Kuveždić3, Martina Dragičević1, Helmuth Berger4, Xavier Rocquefelte5, Mirta Herak1,†, and Tomislav Ivek1

  • 1Institute of Physics, Bijenička cesta 46, 10 000 Zagreb, Croatia
  • 2Faculty of Physics, University of Rijeka, Radmile Matejčić 2, 51 000 Rijeka, Croatia
  • 3Department of Physics, Faculty of Science, University of Zagreb, Bijenička cesta 32, 10 000 Zagreb, Croatia
  • 4Institute of Physics, Ecole Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland
  • 5Univ Rennes, CNRS, ISCR (Institut des Sciences Chimiques de Rennes) UMR 6226, F-35000 Rennes, France

  • *vkisicek@ifs.hr
  • mirta@ifs.hr

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Issue

Vol. 132, Iss. 9 — 1 March 2024

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